Spectroscopy of self-organised “photonic” materials

Supervisor: Dr Ben Murdin


Major Aims:
To investigate completely new 3D “photonic” materials.


Techniques used and source of expertise:
Infrared spectroscopy of novel low-dimensional semiconductor structures. High pressure and high magnetic field spectroscopy of such materials.


Quantum dots are very small islands of semiconductor with very interesting and useful properties, and may be formed spontaneously when depositing epitaxially a very thin layer of the dot material on a substrate of very different lattice constant. In most semiconductor systems they site themselves randomly with large variations in size from dot to dot.

It has recently been shown that quantum dots based on the lead-salt semiconductor system (PbSe on PbEuTe) exhibit a three-dimensional ordering so that the dots arrange themselves in a face-centred cubic array, by Prof. G. Bauer’s group at Linz [G Springholtz et al, Science vol 282, p 734, 1998]. The ordered dot arrays display very high homogeneity in size. So far, there have been no systematic optical studies of these dots.

The subject of "photonic" materials is very similar to X-ray scattering by crystals. It is possible to show that arrays of blobs of material with differing refractive index can set up Bragg scattering in such a way that certain wavelengths of light cannot propagate through the array in any direction, just like the bandgap of a semiconductor. Special defects can be introduced to mimic semiconductor dopants so light can propagate only at a single frequency and in a specific direction. These effects have been demonstrated in the microwave region of the spectrum using mm-scale balls of polystyrene etc etc. This has enormous numbers of technological applications for optoelectronics, if the devices can actually be scaled down in size to optical wavelengths. So far most optical photonic structures are only 2-dimensional. We would like to investigate the possibility of using the self-organised dot material, whose nearest neighbour dot-dot distance is in the optical wavelength regime, as a photonic material.


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